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Entreaty for contributors. Please filter out all purely advertising and non-descriptive epithets like "best", "useful", "handy", "popular", "kick-ass", "professional" and so on.

UI/Theme Frameworks and Components

Ant Design An enterprise-class UI design language and React-based implementation.
Balloon.css Simple tooltips made of pure CSS
Bootflat Open source Flat UI KIT based on Bootstrap
BootPress A PHP Framework with a built in Blog and Flat File CMS
Bootstrap Front-end framework for developing responsive, mobile first projects on the web
Bootswatch Collection of free themes for Bootstrap
Cardinal Small "mobile first" CSS framework for front-end developers who build responsive web applications
Flat UI Free Theme and framework for Bootstrap
Ink set of tools for quick development of web interfaces
Metro UI CSS Set of styles to create a site with an interface similar to Windows 8
Petal A modern, light CSS UI framework developed at Shakr
Pre CSS framework
prelude Lightweight, responsive and extensible front-end framework
Schema Light, responsive, and lean frontend UI framework
Semantic UI UI component framework based around useful principles from natural language
Strapless CSS boilerplate/framework for HTML elements, mixins library for patterns and color
UIkit Lightweight and modular front-end framework for developing web interfaces
ngBoilerplate An opinionated kickstarter for AngularJS projects
Wee Lightweight front-end framework for logically building complex, responsive web projects

Grid Systems

Flexible Grid System
Golden Grid System
Less Zen Grid
Responsive Boilerplate

Mixin Libraries

3L Mixins library
animate Library of CSS3 keyframe animations
Clearless Collection of mixins
Css3LessPlease Conversion of to Less mixins
CssEffects Collection of CSS style effects
Cssowl Mixin library
cube.less Animated 3D cube using only CSS
est Mixin library
Hexagon Generate CSS hexagons with custom size and color
homeless Mixin library
LESS Elements Set of mixins
LESS Hat Mixins library
lessley A jasmine like testing suite written in pure Less
Lessmore Mixins library. Cross-browser support for the CSS3 features and more
LESS-bidi Set of mixins for creating bi-directional styling
LESS-Mix Mixins library
media-query-to-type Media Queries to Media Types with Less
More-Colors.less Variables for easier color manipulation while you design in the browser
more-less Mixin lib supporting Less 1.7
More.less Mixins, animations, shapes and more
more-or-less for-loops and other functions + css3 mixins
normalize.less Modularized famous normalize.css using Less
Oban Collection of mixins
Preboot Collection of variables and mixins. The precursor to Bootstrap
prelude-mixins Collection of mixins
Shape.LESS Collection of mixins for various shapes
tRRtoolbelt.less Mixins and functions for common actions
Tuesday.less CSS Animation mixins library