The verilog project fails under higher clock frequencies (use PLL frequency multiplication 100MHz), and the FPGA output is not as expected

[MisRight]

First of all, this project is really good. I admire you for doing such an excellent job and very interested in your work.
I want to ask you some questions. I tested whether the project works under different system clocks, and found that it can only run normally at 50Mhz or lower frequency. If I use 100Mhz system clock, the output result is unstable or even wrong. How can i solve this problem? I hope to get your guidance, thank you very much anyway.