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guide_spectroscopy.rst

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Nonlinear molecular spectroscopy

  1. Sum-of-states (SOS) for multilevel system

    Pros: computationally cheap and intuitive

    Note

    In the SOS method, decay is introduced phenomelogically.

  2. correlation function approach -- Direct computing the many-point correlation functions with the quantum regression theorem

    Valid for open quantum systems where environment effects can be rigirously described with quantum master equations.

    Visulize with double-sided Feynman diagrams instead of the time-loop diagrams.

  3. non-perturbative approah -- valid for ALL systems provided a quantum dynamics solver is provided.

    Simulating the laser-driven dynamics including explicitly all laser pulses