Description
I cannot find an option to activate the mode bar button for multihover.

Known workarounds
You easily could set the hover mode in the ChartLayout chart |> Chart.withLayout(Layout.init(HoverMode=HoverMode.X)), but the activation of the button would be beneficial for exploratory analyses.
Solution
Addition of hovermode within the ModeBarButton .
open Plotly.NET
[
Chart.Point([1,2])
Chart.Point([1,2])
]
|> Chart.Combine
|> Chart.withConfig(Config.init(ModeBarButtonsToAdd=[ModeBarButton.HoverMode]))
|> Chart.show